It is well known that anisotropy determines the preferred transport direction of carriers. To manipulate the anisotropy is an exciting topic in two-dimensional materials, where the carriers are confined within individual layers. In this work, it is found that uniaxial strain can tune the electronic anisotropy of the 90°-twisted bilayer phosphorene. In this unique bilayer structure, the zigzag direction of one layer corresponds to the armchair one of the other layer and vice versa. Owing to this complementary structure, the directional (zigzag or armchair) deformation response to strain of one layer is opposite to that of the other layer, where the in-plane positive Poisson’s ratio plays a key role. As a result, the doubly degenerate highest valence bands split, followed by a recovery of anisotropy. More interestingly, such an anisotropy, namely, the ratio of the effective mass along the ##IMG## [http://ej.iop.org/images/0295-5075/121/2/…] {$Gamma text{-} X$}

Published in: "EPL".